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Excitation functions of Se(d,xn)Br reactions: Comparative evaluation of possible routes for the production of Br at a small cyclotron
Authors:SM Qaim  G Stcklin
Institution:

Institut für Nuklearchemie, Forschungszentrum Jülich GmbH, D-52425, Jülich, Germany

Abstract:Excitation functions were measured for the first time for 74Se(d,n)75Br and 74Se(d,2n)74mBr reactions from threshold to 23 MeV. Use was made of the stacked-foil technique, and thin samples were prepared by electrolytic deposition of 31.4% enriched 74Se on Al-backing. Differential and integral yields of 74mBr and 75Br were calculated from the measured excitation functions. The optimum energy range for the production of 75Br via the 74Se(d,n)-process was found to be Ed = 12 → 8 MeV, with 75Br-yield amounting to 509 MBq (13.75 mCi)/μAh and the 74mBr impurity to 78Kr(p,greek small letter alpha)75Br and 74Se(d,n)75Br, suggested for the production of 75Br at a small cyclotron is given. The (d,n) reaction gives higher yield than the (p,greek small letter alpha) process and is preferable at cyclotrons with Ed greater-or-equal, slanted 10 MeV. In general, at a small cyclotron the achievable batch yields of 75Br via both the processes are limited.
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