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1.
Purpose: To examine the microdistribution of natural α‐radioactivity in deciduous teeth of children and the permanent teeth of juveniles extracted for orthodontic purpose from across the UK.

Materials and methods: The microdistribution of 210Pb‐supported 210Po and 226Ra in 708 deciduous and permanent teeth and 32 foetal teeth was measured on 1442 TASTRAK α‐particle track detectors.

Results: Of the various findings, a number are of special interest. Around half of the 210Pb activity in the outer enamel of deciduous teeth appears to have been acquired in utero as a result of transplacental transfer. In deciduous and permanent teeth, 226Ra is concentrated mainly in the circumpulpal region, while the highest levels of 210Po are on the highly calcified outer enamel surface. Furthermore, activity concentrations recorded on this surface were ln‐normally distributed.

Conclusions: 210Pb‐supported 210Po activity on the outer enamel surface of permanent teeth constitutes an assay of cumulative environmental exposure with which to assess exposure in bone, both in utero and in childhood. Such assessment can be used to study geographical variations in the α‐activity in teeth. More work is also required to determine the concentrations of both 210Po and 210Pb in the foetal skeleton.  相似文献   

2.
Purpose: To study geographical variations in the level of naturally occurring 210Pb‐supported 210Po in permanent teeth of juveniles in the UK.

Materials and methods: Permanent teeth extracted from 278 juveniles for orthodontic purposes were obtained from 48 counties in the UK. 210Po activity concentration was measured on the outer enamel surface using TASTRAK α‐particle‐sensitive plastic track detectors.

Results: Geometric mean±SE activity concentrations in teeth from urban, suburban and rural areas, excluding the high radon area of Devon, were 8.41 +0.25/?0.24, 7.76 +0.37/?0.35 and 7.20 +0.49/?0.46?Bq?kg?1, respectively. Overall, there was no significant association between α‐activity on the outer enamel surface of permanent teeth and proximity to the major UK motorways. However, when the data were considered with respect to the prevailing south‐westerly wind on the western side of the UK, a statistically significant association with respect to donors living downwind (on the easterly side) of the motorways was found. This effect was greater for sections of the M5 and M6 motorways that traverse urban areas. 210Po levels in teeth were also associated with domestic radon concentration. This effect was comparable with that from traffic and urban pollution.

Conclusions: Higher levels of 210Pb‐supported 210Po are seen in permanent teeth of juveniles near sources of increased exposure in the UK. Inhalation uptake is an important pathway of exposure, especially with respect to domestic radon exposure. The results might be important in assessing integrated exposure to 210Po in the skeleton and consequent high linear energy transfer dose to bone marrow.  相似文献   

3.
PURPOSE: To examine the microdistribution of natural alpha-radioactivity in deciduous teeth of children and the permanent teeth of juveniles extracted for orthodontic purpose from across the UK. MATERIALS AND METHODS: The microdistribution of 210Pb-supported 210Po and 226Ra in 708 deciduous and permanent teeth and 32 foetal teeth was measured on 1442 TASTRAK alpha-particle track detectors. RESULTS: Of the various findings, a number are of special interest. Around half of the 210Pb activity in the outer enamel of deciduous teeth appears to have been acquired in utero as a result of transplacental transfer. In deciduous and permanent teeth, 226Ra is concentrated mainly in the circumpulpal region, while the highest levels of 210Po are on the highly calcified outer enamel surface. Furthermore, activity concentrations recorded on this surface were In-normally distributed. CONCLUSIONS: 210Pb-supported 210Po activity on the outer enamel surface of permanent teeth constitutes an assay of cumulative environmental exposure with which to assess exposure in bone, both in utero and in childhood. Such assessment can be used to study geographical variations in the alpha-activity in teeth. More work is also required to determine the concentrations of both 210Po and 210Pb in the foetal skeleton.  相似文献   

4.
Studies of naturally occurring radioactive materials (NORM) distribution of 226Ra, 228Ra and 40K in East Malaysia were carried out as part of a marine coastal environment project. The results of measurements will serve as baseline data and background reference level for Malaysia coastlines. Sediments from 21 coastal locations and 10 near shore locations were collected for analyses. The samples were dried, finely ground, sealed in a container and stored for a minimum of 30 days to establish secular equilibrium between 226Ra and 228Ra and their respective radioactive progenies. They were counted using a high-purity germanium (HPGe) spectrometer covering the respective progeny energy peak. For 40K, the presence of this was measured directly via its 1460 keV energy peak. The concentration of 226Ra, 228Ra and 40K in samples obtained from coastal Sarawak ranged between 23 and 41 (mean 30±2) Bq/kg, 27 and 45 (mean 39±4) Bq/kg and 142 and 680 (mean 462±59) Bq/kg, respectively. Meanwhile, the concentration of 226Ra, 228Ra and 40K for samples obtained from coastal Sabah ranged between 16 and 30 (mean 23±2) Bq/kg, 23 and 45 (mean 35±4) Bq/kg and 402 and 842 (mean 577±75) Bq/kg, respectively. For the Sarawak near shore stations, the concentration of 226Ra, 228Ra and 40K ranged between 11 and 36 (mean 22±2) Bq/kg, 21 and 65 (mean 39±5) Bq/kg and 149 and 517 (mean 309±41) Bq/kg, respectively. Meanwhile, the concentration of 226Ra, 228Ra and 40K for samples obtained from Sabah ranged between 9 and 31 (mean 14±2) Bq/kg, 10 and 48 (mean 21±3) Bq/kg and 140 and 580 (mean 269±36) Bq/kg, respectively. The calculated external hazard values of between 0.17 and 0.33 (less than unity) showed that there is little risk of external hazard to the workers handling the sediments.  相似文献   

5.
目的 为了解天然放射性核素226Ra、228Ra、210Pb与210Po在水生物及食物链中转移和蓄积情况。方法 定点采集养殖水产品及栖息环境中水与底质沉积物, 按不同的实验需要, 每个鲜样分别剥取肉, 骨(壳),鳞片和胃肠。烹饪样品, 洗净、称重、清炖, 熟后分离出骨(壳),余为食物。样品分别测定226Ra、228Ra、210Pb和210Po含量。数据按统计学要求处理, 配对数据, 作了配对显着性检验。结果 226Ra、228Ra和210Pb主要沉积于骨(壳)中, 浓集系数为102~103,肉中为100~102.210Po主要蓄积在水生物胃肠中, 浓集系数在102~104,鱼类胃肠与贝类肉中可达104.水产食品烹饪加工过程226Ra、228Ra和210Pb在食物链中转移不明显, 经配对显着性检验, 差异无显着性(P0.05);然而210Po在淡水鱼类和虾类中转移是明显的, 肉配对检验有非常显着性差别(P<0.01).结论水生物对226Ra、228Ra、210Pb和210Po有很强浓集能力。  相似文献   

6.
PURPOSE: To study geographical variations in the level of naturally occurring 210Pb-supported 210Po in permanent teeth of juveniles in the UK. MATERIALS AND METHODS: Permanent teeth extracted from 278 juveniles for orthodontic purposes were obtained from 48 counties in the UK. 210Po activity concentration was measured on the outer enamel surface using TASTRAK alpha-particle-sensitive plastic track detectors. RESULTS: Geometric mean +/- SE activity concentrations in teeth from urban, suburban and rural areas, excluding the high radon area of Devon, were 8.41 + 0.25/-0.24, 7.76 + 0.37/-0.35 and 7.20 +0.49/-0.46 Bq kg(-1), respectively. Overall, there was no significant association between alpha-activity on the outer enamel surface of permanent teeth and proximity to the major UK motorways. However, when the data were considered with respect to the prevailing south-westerly wind on the western side of the UK, a statistically significant association with respect to donors living downwind (on the easterly side) of the motorways was found. This effect was greater for sections of the M5 and M6 motorways that traverse urban areas. 210Po levels in teeth were also associated with domestic radon concentration. This effect was comparable with that from traffic and urban pollution. CONCLUSIONS: Higher levels of 210Pb-supported 210Po are seen in permanent teeth of juveniles near sources of increased exposure in the UK. Inhalation uptake is an important pathway of exposure, especially with respect to domestic radon exposure. The results might be important in assessing integrated exposure to 210Po in the skeleton and consequent high linear energy transfer dose to bone marrow.  相似文献   

7.
Purpose:?To study the natural radionuclides in the freshwater fish samples around the uranium mining areas of Bagjata and Banduhurang, East Singhbhum, Jharkhand, India

Materials and methods:?The naturally occurring radioisotopes of uranium, U(nat), consisting of 234U, 235U and 238U; 226Ra, 230Th and 210Po were analysed in the fish samples from the surface water of Bagjata and Banduhurang mining areas after acid digestion. The ingestion dose, concentration factor and excess lifetime cancer risk of the radionuclides were estimated.

Results:?The geometric mean activity of U(nat), 226Ra, 230Th and 210Po in the fish samples was found to be 0.05, 0.19, 0.29 and 0.95 Bq kg?1fresh (Becquerel per kilogram fresh fish), respectively, in the Bagjata mining area, while for Banduhurang mining area it was estimated to be 0.08, 0.41, 0.22 and 2.48 Bq kg?1fresh, respectively. The ingestion dose was computed to be 1.88 and 4.16?μSvY?1, respectively, for both the areas which is much below the 1 mSv limit set in the new International Commission on Radiological Protection (ICRP) recommendations. The estimation of the Concentration Factors (CF) reveal that the CF from water is greater than 1 l/kg?1in most of the cases while from sediment CF is less than 1. The excess individual lifetime cancer risk due to the consumption of fish was calculated to be 2.53?×?10?5 and 6.48?×?10?5, respectively, for Bagjata and Banduhurang areas, which is within the acceptable excess individual lifetime cancer risk value of 1?×?10?4.

Conclusion:?The study confirms that current levels of radioactivity do not pose a significant radiological risk to freshwater fish consumers.  相似文献   

8.
The standard ASTM method is the most commonly applied method for determining 222Rn in drinking water. The method is calibrated with a 226Ra standard solution that usually contains variable amounts of 210Pb, 210Bi and 210Po if the standard has not recently been purified. Until now it has not been experimentally confirmed that these progenies do not interfere when the method is calibrated. In this study, interference was examined using three different organic cocktails and α/β liquid scintillation spectrometry to separately assess the effect of three radionuclides. The interference from 210 Po was 4% for one of the cocktails if the 226Ra standard had been purified 5 years earlier. The interferences from 210Pb and 210Bi were negligible compared to that of 210Po.  相似文献   

9.
目的 调查云南省部分地区大米和玉米放射性核素水平,充实云南地区食品放射性水平基线数据,评估其对居民产生的健康风险。方法 依据国家标准《生物样品中放射性核素的γ能谱分析方法》《高纯锗γ能谱分析通用方法》《食品中放射性物质检验总则》《土壤中放射性核素的γ能谱分析方法》,对云南省20个县(区)大米和玉米样品进行放射性核素检测,对检测结果进行处理与分析。结果 大米样品中238U、232Th、226Ra、40K和137Cs活度浓度均值分别为(0.416±0.403)、(0.045±0.034)、(0.030±0.013)、(28.4±18.8)和(0.014±0.019)Bq/kg,玉米样品中238U、232Th、226Ra、40K活度浓度均值分别为(0.308±0.230)、(0.035±0.031)、(0.053±0.072)、(56.8±38.6)Bq/kg,137Cs的活度浓度低于探测下限。结论 云南省20个县(区)大米和玉米中238U、232Th、226Ra、40K和137Cs的放射性水平均在国家标准正常范围内,食入后不会对居民的健康造成影响。  相似文献   

10.
An analytical method for determination of 210Pb, 226Ra and 228Ra is presented based on adsorption on 3M Empore RadDiscs, and measurement applying liquid scintillation spectrometry (LSC) after elution. The LSC measurement was performed with optimized α⧸β-discrimination and isotope standardization using the triple to double coincidence ratio (TDCR). The consistency of measurement results between radioactive parent–daughter pairs 210Pb/210Bi, 226Ra/222Rn and 228Ra/228Ac was checked in long-term counting experiments and the influence ofinterference of in-growing daughters from 226Ra into the β-spectrum of 228Ra+228Ac was studied as well. Recommendations for optimized LSC 228Ra measurement besides presence of 226Ra are given.  相似文献   

11.
An easy and accurate method for the determination of 210Pb and 210Po in water using 210Po spontaneous deposition onto a silver disk is proposed and assessed for its detection capabilities according to the ISO Guide for the expression of uncertainty in measurement (GUM) and ISO Standard 11929-7 concerning the evaluation of the characteristic limits for ionizing radiation measurements. The method makes no assumption on the initial values of the activity concentrations of 210Pb, 210Bi and 210Po in the sample to be analyzed, and is based on the alpha spectrometric measurement of 210Po in two different aliquots: the first one measured five weeks after the sampling date to ensure radioactive equilibrium between 210Pb and 210Bi and the second after a sufficient time for the ingrowth of 210Po from 210Pb to be significant. As shown, for a recommended time interval of seven months between 210Po measurements, the applicability of the proposed method is limited to water samples with a 226Ra to 210Pb activity ratio CRa/CPb≤4, as usual in natural waters. Using sample and background counting times of 24 h and 240 h, respectively, the detection limit of the activity concentration of each radionuclide at the sampling time for a 1 L sample typically varies between 0.7 and 16 mBq L−1 for 210Pb in water samples with an initial activity of 210Po in the range 0-200 mBq L−1, and between 0.6 and 8.5 mBq L−1 for 210Po in water samples with an initial activity of 210Pb in the same range.  相似文献   

12.
The radon emanation method was applied to measure the activity of 226Ra, dissolved and associated with suspended solids, in the ground waters from two wells drilled in the Morungaba Batholith fractured granites, intruded in the metamorphic basement, eastern border of the Paraná basin in São Paulo State, Brazil. The water samples were collected from March 2003,to April 2004, with a time interval of about one month between sampling campaigns. The mean observed dissolved 226Ra activity concentrations in the two wells were 47.9±7.1 and 51.6±8.8 mBq/L. No systematic time dependence of the 226Ra activity concentration was clearly identified. The activity of 226Ra associated with suspended solids contained in 1 L of ground water fell, during the sampling period, from 13±1 to 0.8±0.1 mBq in one well and from 4.9±0.3 to 0.6±0.1 mBq in the second well.  相似文献   

13.
In the present work, activity concentrations of 222Rn in air and 222Rn and 226Ra in drinking water were measured in Damascus city covering its old and modern parts.It was found that the average air radon activity concentration in the old part was higher than in the modern part, and in drinking water, radon was found to be 60±3 Bq/l, and less than 0.13 Bq/l for radium, which were lower than the recommended levels set by WHO.  相似文献   

14.
Hokutolite consists of barite (BaSO4) and anglesite (PbSO4), and contains significant amounts of radium isotopes as a radioactive mineral. Photon activation and gamma-ray spectrometry were employed to determine Ba, Pb and 226Ra contents in hokutolite samples and to investigate the correlation between 226Ra activity and both Ba and Pb content. 226Ra activity in 30 hokutolite samples were estimated in the range of 40–65 Bq/g and was positively related to Ba content (r=0.859, p<0.001), but independent of Pb content (r=−0.236, p=0.217). Experimental results implied that 226Ra preferably precipitated with Ba over Pb. The 226Ra activity in hokutolite from the Peitou Hot Spring was experimentally estimated based on the Ba/Pb ratio and expressed as 226Ra (Bq/g)=14.67 (Ba/Pb)molar+14.13.  相似文献   

15.
Direct liquid scintillation (LS) methods are widely used for surveying 222Rn in drinking water. Two direct methods are used that differ in sample composition. In a two-phase sample, water lies below a water-immiscible cocktail, while in a homogeneous sample water is mixed with an emulsifying cocktail. Although these methods were developed in the late 1970s, their performances have not been simultaneously tested. Here, the methods were compared in two ways: by preparing both types of sample similarly from 222Rn-bearing groundwater in one emulsifying and in three organic cocktails, and by calibrating the methods with a 226Ra standard according to their respective procedures. The samples were measured using α/β LS spectrometry. The standard deviations of parallel samples and the repeatability of the measurements were excellent for both methods, except two-phase 226Ra samples, whose efficiencies decreased slightly over time. This instability was due to interference from 210Pb, 210Bi and 210Po, which accumulated in the 226Ra standard, and possibly also to the migration of 214Pb and 214Bi into the aqueous phase and deficient transfer of 222Rn from the water to the cocktail.  相似文献   

16.
Measurements of natural radioisotopes present in some of the foodstuffs which form the main components of the composite Indian diet are presented. Assessment of daily intake of these natural radionuclides has been made on the basis of the average daily intake of these food-items by the population of Bombay and its environment. The content of 40K, 226Ra and 228Th radioactivity varies from 45.9 to 649.0 Bq/kg, 0.01 to 1.16 Bq/kg and 0.02 to 1.26 Bq/kg, respectively. The average daily intakes of 40K, 226Ra and 228Th have been estimated as 105.6, 0.17 and 0.18 Bq d−1, respectively for the period 1970–1982.  相似文献   

17.
Summary

Understanding how cellular damage produced by high-linear energy transfer (LET) radiation interacts with that produced by low-LET is important both in radiation therapy and in evaluating risk. To study such interactions, rat lung epithelial cells (LEC) were grown on Mylar® films and exposed to both X-rays and α-particles, separately or simultaneously. Cell killing, and the numbers of binucleated cells and micronuclei, were measured as indicators of damage. X-rays and α-particles given separately caused dose-related increases in cell cycle time, with α-particles producing greater mitotic delay than X-rays. Damage from α-particles and X-rays given simultaneously did not interact to alter further the cell cycle. Cell survival data following exposure to X-rays and α-particles, combined or individually, were fitted by linear-quadratic models. Survival curves following exposure to α-particles only, or to 1·0 Gy α-particles plus graded X-ray doses, were adequately described using only the linear (α) term of a linear-quadratic model with α coefficients of 0·9 ± 0·04 and 1·03 ± 0·18 Gy?1, respectively. Survival following exposure to X-rays only or to 0·06 Gy α-particles combined with X-rays was best fitted using both α and β terms of the linear-quadratic model (0·12 ± 0·03)D + (0·007 ± 0·002)D2 and (0·57 ± 0·08)D + (0·3 ± 0·02)D2, respectively. The numbers of micronuclei produced by exposure to α-particles or X-rays alone increased linearly with dose, with slopes of 0·48 ± 0·07 and 0·19 ± 0·05 micronuclei/binucleated cell per Gy for α and X-rays, respectively. Simultaneous exposure to graded levels of X-rays and a constant α dose of either 1·0 or 0·06 Gy increased micronuclei frequency, with a slope of 0·74 ± 0·05 or 0·58 ± 0·04 micronuclei/binucleated cell per Gy, respectively. These slopes are similar to that produced by α-particles alone. These studies demonstrated that both cell killing and the induction of micronuclei were increased by combined exposure compared with that predicted for separate exposures.  相似文献   

18.
The measurements of gross alpha and gross beta radioactivity in groundwater samples from Guarani aquifer in Brazil are reported in this paper together with the activity concentration of the natural dissolved radionuclides (40)K, (238)U, (234)U, (226)Ra, (222)Rn, (210)Po, (210)Pb, (232)Th, (228Th), and (228)Ra. Most of the gross alpha radioactivity values were below the critical level of detection corresponding to 1mBq/L, however, the whole data set for the gross beta radioactivity and radionuclides (40)K, (238)U, (234)U, (226)Ra, (222)Rn, (210)Po, (210)Pb, and (228)Ra was submitted to a statistical treatment, considering class intervals arranged in geometric progression, because of the great variability of the activity. The analysis indicated lognormal distribution of the data, as usually observed in samples taken from the natural context. An inverse relationship between the gross alpha and gross beta activity has been identified and is related to an increase in the K content in the water. The mobility coefficient has been estimated for (238)U, (226)Ra, (232)Th and (228)Ra in Guarani aquifer and the results indicated that the radioelement solubility in the studied system varies according to the following order: radium>uranium>thorium. The implications of the data obtained in terms of standards established for defining the drinking water quality have also been discussed.  相似文献   

19.
Summary

The induction of bone cancer in mice, dogs and humans, due to protracted α-irradiation from skeletal burdens of radium, was found to be represented by a single dose-rate/time/response function, when time was normalized with respect to species natural life-span. In the absence of other causes of death, the median time to death from bone cancer after 226Ra intake is given by t*m = 790d¯* ? 0·29, based on the dog data, with d¯* the time-weighted average absorbed dose rate in cGy/mLSF to skeleton and where time is measured as milli-life-span-fraction. On the basis of life-span scaling of the time dimension, data on cancer induction from studies with laboratory animals can be scaled to estimate human risks in a three-step process involving a three-dimensional analysis. The overall cancer risk distribution is shown to be a mountain-like surface rising from a Euclidean plane formed by the dose rate and survival time co-ordinates. At lower dose rates the time required for cancer induction may exceed the natural life-span yielding a quasi-threshold for cancer risk. For intakes of 226Ra in young adults this quasi-threshold is predicted to occur at a cumulative life-time α-radiation dose to the skeleton of about 1 Gy.  相似文献   

20.
In this paper, the 222Rn and 226Ra activity concentration was measured in groundwater samples collected from the Bauru Aquifer System, São José do Rio Preto city, São Paulo State, Brazil. The site has been selected for a detailed radiometric survey due to the large number of tubular wells drilled in the aquifer there, which provide water for ~70% of the local population. Despite the importance of groundwater for the local water-supply system, there is a lack of both 222Rn and 226Ra data in the municipality. Establishment of these data is relevant to assure that the water quality from a radiological point of view, is not health threat. São José do Rio Preto city is geologically situated in Bauru Group that is located within the Paraná sedimentary basin. The monitoring program involved the collection of 50 groundwater samples from deep tubular wells during three field campaigns held from 17th to 19th January 2011, from 2nd to 3rd August 2011 and in 30th November 2011. Temperature and pH readings were realized in the field, whereas 222Rn and 226Ra analysis were performed at the laboratory using the Alpha Guard-Aquakit analytical protocol, which allowed us to obtain 222Rn activity concentration ranging from 0.69 to 14.95 Bq/L. These data indicate that the abundances of 222Rn and 226Ra in the groundwater system of Bauru Group is below the WHO guideline limit of 100 Bq/L. Chemical analysis has been also realized for major cations and anions in order to better understand the water features in the municipality.  相似文献   

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