Estimation of the radiological risk related to the presence of radon 222 in a hydrotherapy centre in Tunisia.

The (222)Rn concentration in air was measured in a thermal water spa used as a hydrotherapy centre in Tunisia. The associated health risk for employees and patients due to the inhalation of (222)Rn and its progeny was estimated. A protection scheme for the employees of the spas has been designed. Results show that the (222)Rn concentration varies in the range 33-589 Bq m(-3). The (222)Rn concentrations measured in the present study show lower values in comparison to those reported for thermal spas in other countries. The (222)Rn concentration in different rooms of the spa depends mainly on the ventilation rate. A model based on a dosimetric approach was adopted to estimate the radon risk considering the (222)Rn concentration, the time spent in the spa, and the radioactive equilibrium factor F. The annual effective dose was found to vary between 0.2 and 1.7 mSv for workers while the range for patients was from 2.8 x 10(-4) to 1.1 x 10(-4) mSv. These values are within the ICRP recommended values.     

222Rn air concentration and radiation exposure levels in the Lantian Xishui karst cave of Shaanxi, China

22Rn air concentrations in the Lantian Xishui karst cave of Shaanxi, China, were measured by continuous monitoring during a complete annual cycle (March 2004-February 2005) and annual doses for tour guides and visitors were estimated. The 22Rn air concentrations in the cave vary between a minimum of 383.6 Bq m(-3) and a maximum of 2,015.7 Bq m(-3), with an annual average of 1,100.4 Bq m(-3). Distinct seasonal variation of radon air concentrations inside the cave was observed. The maximum average radon concentration occurred in summer and the minimum average radon concentration occurred in winter. The annual effective dose to tour guides varies between an average of 1.2 mSv and 4.9 mSv depending on different equilibrium factors together with different dose conversion factors proposed in the literature, which is lower than the international recommendations. In all cases, the annual effective doses to visitors are well under the 1 mSv maximum suggested dose for a member of the public for one year.     

崇明县空气中氡浓度水平调查与评价

目的 了解崇明县室内外氡浓度水平并估算其所致公众的受照剂量。方法 根据2010年全国人口普查崇明县乡镇人口比例、房屋建筑类型、建筑年代和主体建筑材料等对测量样本进行分类选择。使用美国Durridge公司制造RAD7型电子氡气检测仪对室内外氡进行测量,数据采用SPSS 17.0软件进行统计分析。结果 本次调查的室内²²²Rn浓度范围为5.75~195.29 Bq/m³,平均浓度为(25.76±2.07) Bq/m³。约有73.89%的房屋内氡浓度低于40 Bq/m³。室外²²²Rn浓度的范围为5.70~19.32 Bq/m³,平均浓度为(9.92±1.43) Bq/m³。结论 本次调查的崇明县室内氡浓度均未超过国家推荐的控制限值。崇明县居民吸入氡所致人年均有效剂量为0.74 mSv。     

Micrometer-sized short-lived radioactive aerosol particles for convenient use in laboratory measurements

For calibration and testing of radioactive aerosol measuring equipment such as continuous air monitors and cascade impactors, and other research applications, it is helpful to have a convenient and relatively safe means of producing radioactive aerosol particles of controlled size and activity. We describe a technique for producing such particles in the micrometer-diameter size range using electrostatic deposition of radon decay products onto otherwise nonradioactive powders of different sizes. An electric field focuses radon decay products (primarily 218Po) onto the surface of a powdered substrate that is then suspended by a technique such as pneumatic dry dispersion. Only a modest-activity commercial 222Rn source (e.g., containing as little as 10(5) Bq of 226Ra) is required, and issues of radioactive cleanup and contamination are minimized due to the short half-lives (26.8 min or less) of the decay products. We report representative results using powders of glass beads, iron oxide, and iron and gold metals in the size range of 0.3 to 30 microm. Yields for the deposited radioactivity per unit concentration of 222Rn gas were of the order of 5 x 10(-7) Bq (214Bi) per milligram substrate per Bq m(-3) of 222Rn for an electrostatic collection time of 30 min.     

An instrument for measuring equilibrium-equivalent 222Rn and 220Rn concentrations with etched track detectors.

To simultaneously measure both 222Rn and 220Rn progeny concentrations, a new type of portable integrating monitor with allyl diglycol carbonate (CR-39) plastic detectors was developed. The monitor gives the average equilibrium-equivalent 222Rn and 220Rn concentrations (EEC(RN) and EEC(Tn)) during sampling intervals. The detection efficiencies of the alpha particles were calculated by Monte Carlo method. The lower limits of detection for EEC(Rn) and EEC(Tn) are estimated to be 0.57 Bq m(-3) and 0.07 Bq m(-3) for 24 h continuously sampling at a flow rate of 0.8 L min(-1). The measuring results with the new type monitors were confirmed through intercomparison experiments. In a small survey, a rather high 220Rn progeny concentration with an average of 1.73 Bq m(-3) was observed in traditional Japanese dwellings with soil/mud plastered walls. On the other hand, a very high 232Th concentration in soil was reported in China. They suggested that there is a possibility of high 220Rn progeny concentration in both Japan and China.     

Radon in a self-selected sample of Israeli homes, schools, and workplaces.

Some 1,100 residences and places of work and 400 schoolrooms in Israel were tested for ambient air radon activity concentration in response to requests by the owners, tenants, or local authorities. A polyethylene vial containing activated charcoal was exposed to room air in each of these structures for 7 days, sealed, and transported to the laboratory. Adsorbed radon was extracted with a toluene-based cocktail which was then subjected to liquid scintillation counting. Mean radon activity concentrations were found to vary from city to city by more than an order of magnitude, indicating strong regional differences. The countrywide geometric mean was found to be 38 Bq/m3; the median, 37. The range for these means was 6-77 Bq/m3; for the medians, 11-100 Bq/m3. The highest reading was 9,100 Bq/m3. Our results are basically in line with those from the United States and much of Europe, but apparently higher than those found in the United Kingdom and Japan. It may be fairly said that mass testing for radon (222Rn) inside buildings in the United States began in the wake of the finding of a radon activity concentration in excess of 100,000 Bq/m3 in the home of the Watras family in Boyertown, PA in December 1984. To date, literally millions of American buildings have been tested, and mandatory testing of schoolrooms has begun in some states. In Israel, by contrast, where such a dramatically high measurement has not (yet) occurred, only 5 structures had been checked for radon by 1989.(ABSTRACT TRUNCATED AT 250 WORDS)     

Seasonal variation in indoor radon concentrations in dwellings in six districts of the Punjab province, Pakistan

An indoor radon measurement survey has been carried out in six districts of the Punjab province. These included Gujranwala, Gujrat, Hafizabad, Sialkot, Narowal and Mandibahauddin districts. In each district, 40 representative houses were chosen and indoor radon levels were measured in these dwellings in autumn, winter, spring and summer seasons using CR-39 based NRPB radon dosimeters. After exposure to radon, the CR-39 detectors were etched in 25% NaOH at 80 degrees C and track densities were related to radon concentration levels. From the observed data, average radon concentration levels and a seasonal correction factor were calculated. The average 222Rn concentration level was found to vary from 40 +/- 15 to 160 +/- 32 Bq m(-3) and 38 +/- 17 to 141 +/- 26 Bq m(-3) in the bedrooms and living rooms of the houses surveyed, respectively. The annual mean effective dose received by the occupants has been calculated using ICRP (1993 Ann. ICRP 23) and UNSCEAR (2000 Sources and Effects of Ionizing Radiation (New York: United Nations)); it varied from 1.2 to 1.7 mSv and from 1.8 to 2.4 mSv, respectively.     

汕头市环境中氡水平及所致居民剂量的分析

本文报道了汕头市室内外环境中氡土气浓度及其子体潜能浓度。研究结果显示：本市环境天然辐射水平较高,室内外氡浓度分别为２００４、１６０５Ｂｑ／ｍ３,土气浓度分别为４１８５、３１１５Ｂｑ／ｍ３,氡子体分别为０００２５４、０００２６８ＷＬ,土气子体分别为０００３３１、０００２４５ＷＬ。汕头市居民吸入氡土气及其子体所致的年有效剂量当量为１２６ｍＳｖ,其中２２２Ｒｎ及其子体贡献了０９０３ｍＳｖ,即氡及其子体所贡献的年有效剂量当量占７５％,较接近于温带地区而高于全球正常本底地区（０９７ｍＳｖ）的水平     

Quality control of mitigation methods for unusually high indoor radon concentrations

The present study's objective was to control the quality of different mitigation methods for unusually high indoor radon (222Rn) concentrations of up to 274,000 Bq m(-3) in a village (Umhausen, 2,600 inhabitants) in western Tyrol, Austria. Five years after mitigation, five different remedial actions were examined on their quality by means of measuring indoor radon concentrations with charcoal liquid scintillation radon detectors and with a continuously recording AlphaGuard detector. Mitigation method in house 1--a mechanical intake and outlet ventilation system with heat exchanger in the basement, combined with a soil depressurization system--was characterized by long-term stability. With most favorable air pressure (+100 Pa) in the basement, mean basement radon concentrations in the winter were reduced from 200,000 Bq m(-3) to 3,000 Bq m(-3) by this method 5 y after mitigation. Acting against experts' instructions, the inhabitants had switched off the ventilation system most of the time to minimize power consumption although it had been proven that ventilation reduced mean basement radon concentration by a factor of about 3 in the winter and about 15 in the summer. Mitigation method in house 2-soil depressurization with two fans and loops of drainage tubes to withdraw radon from the region below the floor and outside the basement walls, and from soil below that part of the house with no basement-had been the most successful remedial measure until the winter of 1999 (i.e., 6 y after mitigation), when micro-cracks opened and consequently mean basement radon concentration increased from 250 Bq m(-3) to 1,500 Bq m(-3). Measures to block these microcracks and to minimize soil drying are being developed. Five years after mitigation, the remedial method used in house 3--a multilayer floor construction, where a fan was used to suck radon from a layer between bottom slab and floor-reduced winter mean radon concentration from 25,000 Bq m(-3) to 1,200 Bq m(-3), with the ventilation on and the basement door open. Mitigation method in house 4--a basement sealing technique--was unsuccessful with almost identical radon concentrations during all the five years since mitigation had started. Mitigation method in house 5--a waterproof basement technique especially for future homes--reduced mean basement radon concentration below 300 Bq m(-3) and mean ground floor radon concentration below 200 Bq m(-3), which is the Austrian action level for newly constructed buildings. These findings indicate that even in areas with extremely high radon concentrations, effective mitigation of indoor radon can be achieved provided that house-specific long-term, stable mitigation techniques are applied.     

Indoor radon in the region of Brussels

The indoor radon (222Rn) concentration has been measured by charcoal detectors in 278 buildings in the region of Brussels, Belgium. The correlation with the nature of the subsoil can be studied in detail thanks to the available geotechnical map. With a geometrical mean indoor radon concentration of 19 Bq m(-3), Brussels can be considered as generally unaffected by the radon problem. No value higher than 400 Bq m(-3) (the EU reference level for existing houses) was measured in an occupied room. However, two factors that may enhance the risk are identified: the absence of a basement or a ventilated crawl space, and the presence of loess, under the house. About one third of the houses without basements or ventilated crawl spaces built on loess show an indoor radon concentration above 200 Bq m(-3) (the EU reference level for new houses).     

名古屋市室内空气222Rn、220Rn的测量及EECTn估算

目的 研究室内空气中^222Rn、^220Rn浓度以及室内平衡当量^220Rn浓度EECTn。方法 利用名古屋大学研制的新型被动累积式^222Rn、^220Rn测量杯在日本名古屋市进行了小规模的室内^222Rn、^220Rn的浓度调查，利用Deposition Rate Monitor估算了住宅室内EECTn。结果 在随机抽查的20个住宅室内^222Rn平均浓度为16．94Bqm^-3；其中5个住宅室内^220Rn平均浓度为58．09Bqm^-3，EEGTn平均值为2．75Bqm^-3。结论 本研究结果与日本全国性调查结果^222Rn浓度平均值15．5Bqm^-3相当。^220Rn的浓度在某些泥土墙壁的住房内可能达到比较高的浓度，进行进一步的研究是很有必要的。     

Preliminary experiences with 222Rn gas in Arizona homes

Results of a survey of 222Rn gas using four-day charcoal canister tests in 759 Arizona homes are reported. Although the study was not random with respect to population or land area, it was useful in identifying areas at risk and locating several homes having elevated indoor 222Rn air concentrations. Approximately 18% of the homes tested exceeded 150 Bq m-3 (4 pCi L-1), with 7% exceeding 300 Bq m-3 (8 pCi L-1). Several Arizona cities had larger fractions of homes exceeding 150 Bq m-3 (4 pCi L-1), such as Carefree and Cave Creek (23%), Paradise Valley (30%), Payson (33%), and Prescott (31%). The Granite Dells and Groom Creek areas of Prescott had in excess of 40-60% of the houses tested exceeding 150 Bq m-3 (4 pCi L-1). Elevated 222Rn concentrations were measured for a variety of home types having different construction materials. Private well water was identified as a potentially significant source of 222Rn gas in Prescott homes, with water from one well testing over 3.5 MBq m-3 (94,000 pCi L-1). A 222Rn concentration in air exceeding 410,000 Bq m-3 (11,000 pCi L-1) was measured using a four-day charcoal canister test in a house in Prescott which had a well opening into a living space. Additional measurements in this 150-m3 dwelling revealed a strikingly heterogeneous 222Rn concentration. The excessive 222Rn level in the dwelling was reduced to less than 190 Bq m-3 (5.2 pCi L-1) by sealing the well head with caulking and providing passive ventilation through a pipe.     

Continuous measurements of outdoor 222Rn concentrations for three years at one location in Colorado

Measurements were made of 222Rn concentrations outdoors in Ft. Collins, Colorado, using a continuously sampling scintillation flask between January 1993 and December 1995. These data were analyzed for hourly, daily, and seasonal variations. The average 222Rn concentration at 1 m above the ground was 18 +/- 10 Bq m(-3) with a geometric mean of 15 Bq m(-3) and a geometric standard deviation of 1.7. Hourly averaged data indicated a diurnal pattern with the outdoor 222Rn concentration reaching a maximum in the early morning between 4:00 a.m. and 6:00 a.m. and a broad minimum between 1:00 p.m. and 4:00 p.m. in the afternoon. An analysis also indicated that the outdoor 222Rn concentrations were consistently lowest during the spring (March and April) and highest during the late summer (July-September).     

Spatial variation of waterborne radon and temporal variation of radon in water at nine Maine schools

Nine elementary schools in Maine were examined to track the release of 222Rn and to determine the transfer coefficient from water into air. Water-use simulations were performed by running sinks and sprayers for 1 h in a kitchen. The 222Rn in air was measured over 24 h throughout the school. The subsequent release of 222Rn into the kitchen air was measured to be greater than the EPA action level of 0.15 Bq L-1 (4 pCi L-1), but negligible concentrations of 222Rn were found in adjacent classrooms. In two schools, more than 10 222Rn-in-air detectors were placed throughout the kitchen and showed a three-fold spatial concentration variation. During the hour-long simulations, the 222Rn in water concentration was measured periodically, and many of the schools showed an increase in the 222Rn concentration in water before remaining constant. These measured variations suggest that multiple detectors are needed to accurately measure waterborne 222Rn in air, and multiple delayed measurements of 222Rn dissolved in water are needed to obtain a representative groundwater sample.     

Radon-222 concentrations and decay-product equilibrium in dwellings and in the open air

Results are presented of measurements of the activity concentrations of 222Rn and its short-lived decay products and the 212Pb/212Bi concentrations in more than 200 dwellings in West Germany and in the open air. For more than 130 measurements of the equilibrium factor F in dwellings the median value was found to be 0.3. Measurements of F in the open air under various conditions resulted in a mean value of about 0.4. The results of the investigations showed that indoors F depends only slightly on ventilation, indoor 222Rn concentration and other parameters. The equilibrium factor F in the open air, however, was found to depend on meteorological conditions. Empirical correlations from the data obtained for the daughter/222Rn concentration ratios were derived to provide relations for the prediction of the individual daughter product concentrations at a measured 222Rn level. It was established that the daughter/222Rn concentration ratios for indoor air do not change within the range of 222Rn concentrations investigated (1-370 Bq X m-3). These relations, however, are not valid for the daughter/222Rn concentration ratios in outdoor air. The correlations derived further suggest that the individual daughter product concentrations may be assessed with sufficient accuracy by only measuring the 222Rn concentrations. Thus the daughter ratios obtained in this way should enable good estimates of the lung dose for members of the public due to inhalation of the short-lived 222Rn daughters and the dose contribution of the individual 222Rn-daughter products.     

Radon and thoron in cave dwellings (Yan'an, China)

222Rn and 220Rn concentrations were measured in cave dwellings and brick houses in the region of Yan'an (China) during summer 1997. The underground dwellings are built into Quaternary loess, and all investigated houses are founded on it. The median values of indoor 222Rn and 220Rn concentrations are 42 (n = 18) and 77 Bq m(-3) (n = 15) for brick houses and 92 (n = 23) and 215 (n = 17) Bq m(-3) for cave dwellings. To classify the dwellings in respect to their "cave-character," the fraction of walls having a direct contact to the loses is calculated for each dwelling. While the 222Rn concentrations are increasing with higher fractions, the 220Rn concentrations are not correlated with this fraction. On the other hand, due to the short half-life of 220Rn the distance from the measuring point to the walls is negatively correlated with the 220Rn concentration, while there is no correlation with the 222Rn concentration. Therefore, concentric isolines of 220Rn concentrations showing a strong gradient were detected in cave dwellings. An influence of the ventilation rate is distinct for 222Rn but weak for 220Rn. The effective dose rates for 222Rn and 220Rn and their progenies are calculated for brick houses (2.7 mSv y(-1)), cave dwellings (7.1 mSv y(-1)), and for traditional cave dwellings with a bed foundation built with loess (16.7 mSv y(-1)). These calculations are based on summer measurements only. It is expected that the true effective dose rates will be significantly higher.     

Underground air returns as active transportation pathways for radon gas entry into homes.

Levels of elevated 222Rn in homes can fail to correlate with measured radium concentrations in soils and surrounding rocks for reasons which can include water sources, building materials, and unusual variations in climate or building construction. Several homes were identified in the Phoenix, AZ metropolitan area with soil radium concentrations of < 0.074 Bq g-1 (2.0 pCi g-1) which had elevated radon concentrations unexplained by geological sources alone. Continuous monitoring of eight houses under different conditions of cooling system usage revealed a definite role of the underground air returns as active transport pathways contributing to the enhancement of the indoor concentration of 222Rn in six of the houses. The ratio of indoor 222Rn concentrations on days when the cooling system was operated continuously compared to days the system was off ranged from essentially one up to a factor exceeding 10.     

Correlation among the terrestrial gamma radiation, the indoor air 222Rn, and the tap water 222Rn in Switzerland

The external gamma radiation and the indoor air Rn (222Rn) concentration were measured in 55 houses of the South East Grisons, the Urseren valley, and the Upper Rhine valley (crystalline subsoils) and in 39 houses of the Molasse basin and the Helvetic nappes (sedimentary subsoils). In homes located on a crystalline subsoil, a mean cellar gamma level of 1.40 mGy y-1 was measured, which is twice the mean gamma level of 0.70 mGy y-1 found in homes built on a sedimentary subsoil. The cellar 222Rn gas concentration is about six times higher in houses with a crystalline subsoil (1232 Bq m-3) than in houses with a sedimentary subsoil (201 Bq m-3). Although a weak correlation is observed between the mean gamma radiation levels and mean cellar 222Rn gas concentrations for the five subregions investigated, the gamma levels and the 222Rn gas concentrations do not correlate for single homes. For the population living on the ground floor of a house with a crystalline subsoil, the gamma radiation and the indoor air 222Rn lead to estimated mean exposures of 1.16 mSv and 9.44 mSv effective dose equivalent per year, respectively. In houses with a sedimentary subsoil, these mean exposures lead to 0.68 mSv y-1 and 3.22 mSv y-1, respectively. A mean tap water 222Rn content of 38.3 Bq L-1 and 10.4 Bq L-1 was measured in 31 villages with a crystalline subsoil and 73 villages with a sedimentary subsoil, respectively. Radon-222 degasing from the tap water into the indoor air leads to an additional exposure of about 0.11 mSv y-1 and 0.03 mSv y-1 in homes with a crystalline subsoil and homes with a sedimentary subsoil, respectively.     

Radon in Irish schools: the results of a national survey.

This paper presents the results of a survey of radon concentrations in Irish primary and post-primary schools. The objective of this survey was to assess the distribution of radon in Irish schools and to identify those requiring remedial work to reduce radon exposure to children and staff. All primary and post-primary schools were invited to participate in the survey. Indoor radon concentrations were measured during the academic year using integrating passive alpha track-etch detectors with a measurement period from three to nine months. The survey was carried out on a phased basis from 1998 to 2004 and is one of the most comprehensive of its kind undertaken in Europe. Measurements were completed in 38 531 ground floor classrooms and offices in 3826 schools, representing over 95% of the approximate 4000 primary and post-primary schools in Ireland. Of these, 984 schools had radon concentrations greater than 200 Bq m(-3) in 3028 rooms and 329 schools had radon concentrations in excess of 400 Bq m(-3) in 800 rooms. The average radon concentration in schools was 93 Bq m(-3). This results in an annual average effective dose to an Irish child from exposure to radon of 0.3 mSv per year, assuming that the long-term radon concentration is equal to the radon concentration present during the working hours and that the annual average occupancy is 1000 h per year. A programme of remediation of schools with radon concentrations above 200 Bq m(-3) has been put in place.     

Indoor 222Rn measurements in Sweden with the solid-state nuclear track detector technique

Measurements of the indoor radon and radon daughter concentrations were performed in several thousand Swedish houses during the years 1979-1984 with the solid state nuclear track detector technique (SSNTD technique). The investigation focused on structures containing building materials of light-weight concrete with enhanced amounts of U. The detectors used nuclear track films exposed for 1 mo. The film basically measures total airborne alpha activity but may be calibrated in units of EER in an environment with known 222Rn and daughter concentrations. (EER is here the equilibrium equivalent concentration of Rn with the equilibrium factor F = 0.5.) The investigation was performed in various municipalities in collaboration with the local public health and environmental authorities. The investigation included 6700 individual measurements in detached (single-family) houses as well as in apartment houses. A small percentage of the dwellings exhibited Rn daughter concentrations (EER) exceeding 400 Bq m-3. It was found in detached houses that the concentrations were higher in the basement floor than in the entrance floor of a house. The Rn daughter values in the bedrooms were similar to values in any other room (mainly on the same floor) of the structure. The Rn daughter levels in apartment houses were lower than in single-family houses. The seasonal variations of the Rn daughter levels are presented and show that the levels in summertime are approximately equal to the levels in the winter.