Permeability of caulking compounds to 222Rn.

Caulking compounds have been tested as 222Rn barriers. Of these, the most effective is GE acrylic Latex Silicone Caulk, 0.2 cm of which attenuates 222Rn by 98% to 99.9%. The same thickness of two commercial 222Rn barriers attenuates radon by 75% to 90%. Permeabilities range from 0.3 to 140 x 10(-8) cm2 s-1.     

Quantitative goals for a 222Rn multimedia mitigation plan.

The U.S. Environmental Protection Agency's revised proposed 222Rn in drinking water regulation gives states or individual community water systems the option of compliance with the maximum contaminant level or compliance with the higher, alternate maximum contaminant level accompanied by the implementation of a multimedia mitigation plan. If states or water suppliers choose to comply with the alternate maximum contaminant level, the health risk reduction achieved by multimedia mitigation programs must be equal to or greater than the health risk reduction that would be achieved by compliance with the maximum contaminant level rather than the alternate maximum contaminant level. We have developed a method to determine quantitative goals for mitigating existing homes and building new 222Rn-resistant homes to achieve a health risk reduction to the public equivalent to the health risk differential between alternate maximum contaminant level and maximum contaminant level compliance. This method can be applied to an entire state, a portion of a state, or to an individual water supplier. The method was applied to North Carolina, and it was concluded that, over time, the health risk reduction achievable from alternate maximum contaminant level compliance and the implementation of a multimedia mitigation program would be much greater than from compliance with the maximum contaminant level.     

Contribution of 222Rn in domestic water supplies to 222Rn in indoor air in Colorado homes.

The contribution of 222Rn from domestic water wells to indoor air was investigated in a study of 28 houses near Conifer, CO. Air concentrations determined by alpha-track detectors (ATDs) and continuous radon monitors were compared with the predictions of a single-cell model. In many of the houses, the water supply was shown to contribute significantly to levels of indoor 222Rn. The data from the ATD study were augmented with a continuous monitoring study of a house near Lyons, CO. The well water in that house has the highest known concentration of 222Rn in water yet reported (93 MBq m-3). The temporal pattern in the indoor 222Rn concentration corresponds to water-use records. In general, it is difficult to quantify the proportion of indoor radon attributable to water use. Several lines of evidence suggest that the single-cell model underestimates this proportion. Continuous-monitoring data, although useful, are impractical due to the cost of the equipment. We propose a protocol for 222Rn measurement based on three simultaneous integrating radon detectors that may help estimate the proportion of indoor 222Rn derived from the water supply.     

Gamma distribution and house 222Rn measurements.

The statistical distribution of 222Rn measurements from basements and first floors of homes in northeastern Pennsylvania was investigated. The gamma distribution was statistically significantly superior to the normal distribution (p less than 0.005) in describing the frequency distribution of the logarithm of observed 222Rn levels. The fit to the data was closer both in the central portion and in the upper tail. The gamma distribution has certain characteristics that make it generally useful in the study of environmental toxic agents where several different exposures over a lifetime occur and must be combined, as for risk assessment or for statistical power calculations for epidemiologic studies.     

Developing soil gas and 222Rn entry potentials for substructure surfaces and assessing 222Rn control diagnostic techniques

Research-based procedures for characterizing the causes of elevated indoor 222Rn levels and guiding the selection of an appropriate control technique were evaluated at seven New Jersey houses. Procedures such as thorough visual inspections, blower door air leakage tests, pressure field mapping, subsurface vacuum extension tests, sampling of 222Rn concentrations throughout the substructure, and measurements of the additional depressurization caused by various appliances all were found to furnish important information to the mitigation contractor or researcher. An analysis of data from these and other diagnostic techniques performed at the seven houses also indicated: (1) regions of very high permeability existed directly adjacent to the exterior of substructure walls and floors; (2) the additional substructure depressurization caused by operation of forced-air furnaces and attic exhaust fans could exceed 1 Pascal; (3) 222Rn concentrations below basement slabs and slabs-on-grade adjoining below grade basement walls were approximately seven times higher than those within block wall cavities; and (4) air leakage areas of crawlspace and basement ceilings were quite large, ranging up to 0.15 m2. The pressure field mapping tests identified the areas surrounding the substructure that were well coupled to the indoors. Using flow, pressure difference, and 222Rn concentration data, indices of soil gas entry potential and 222Rn entry potential were developed to indicate the areas of the substructure that may have high entry rates of soil gas and 222Rn, respectively. These indices could be helpful for quantifying the relative resistance to soil gas movement of substructure surfaces and surrounding soils and for determining the placement of 222Rn control systems.     

Study of 222Rn permeation through polymer membranes: application to continuous measurement of 222Rn in water.

Membranes that exclude water but are permeable to radon can extend the range of environments where many radon detection systems could operate. We have studied the permeation of 222Rn through polypropylene membranes separating air and water phases. The permeation coefficient and the activation energy were calculated for various conditions. Potential applications, such as in situ detection of radon in water, are discussed.     

Radon-222, 222Rn progeny, and 220Rn progeny levels in 70 houses

A year-long, multipollutant, indoor air quality study involving 70 occupied houses in four states was completed in 1987. All of the houses included in the study had a partial or complete basement with a concrete slab floor and block walls. On an approximately quarterly schedule, integrating monitors for short-lived Rn progeny, nitrogen dioxide, formaldehyde, and water vapor were exposed for 1 wk in each house on both the basement and main floors. At the beginning of the study, a pair of alpha-track detectors were placed on top of the refrigerator in the kitchen (or some other sampling location on the main floor) and at a location in the basement. One detector at each location was left in place for a year while the other detector was retrieved and replaced once every 3-mo period. In addition, short-term measurements of Rn and 222Rn progeny were made at all sampling locations once per quarter. In this study, comparisons were made between: (1) seasonal and annual averages, (2) summer and winter averages, (3) living-area and basement results, (4) 222Rn and 220Rn progeny, and (5) short- and long-term measurements. The Rn and Rn progeny concentrations in houses near Huntsville, AL were found to be well above recommended action levels (150 Bq m-3). For houses near Birmingham, AL, summer Rn concentrations were found to exceed winter concentrations, whereas for the other houses in the study, winter concentrations exceeded summer concentrations. Potential alpha energy concentrations (PAEC) from 220Rn progeny were found to be generally less than PAEC from 222Rn.     

Multi-state surveys of indoor 222Rn

The U.S. Environmental Protection Agency provides assistance to states in conducting surveys of indoor 222Rn. Alabama, Kentucky, Tennessee, Wisconsin, and Wyoming completed statistically designed surveys during the 1986-1987 heating season. In all states, probability-based samples of 5800 houses were tested using charcoal canisters exposed for 48 h. Thus, sample results can be validly extrapolated to the target population of all owner-occupied, ground-level houses having listed telephone numbers. Estimates of population parameters (e.g., median) and their associated confidence intervals are given for each state, for geographic regions within states, and for basement and nonbasement houses. Results confirm that 222Rn concentration varies widely from one state to another and from one geographic region to another within a state; however, the same pattern of differences was not evident in basement or nonbasement houses. Short-term 222Rn readings appear to follow a log-normal distribution.     

An instrument for measuring equilibrium-equivalent 222Rn and 220Rn concentrations with etched track detectors.

To simultaneously measure both 222Rn and 220Rn progeny concentrations, a new type of portable integrating monitor with allyl diglycol carbonate (CR-39) plastic detectors was developed. The monitor gives the average equilibrium-equivalent 222Rn and 220Rn concentrations (EEC(RN) and EEC(Tn)) during sampling intervals. The detection efficiencies of the alpha particles were calculated by Monte Carlo method. The lower limits of detection for EEC(Rn) and EEC(Tn) are estimated to be 0.57 Bq m(-3) and 0.07 Bq m(-3) for 24 h continuously sampling at a flow rate of 0.8 L min(-1). The measuring results with the new type monitors were confirmed through intercomparison experiments. In a small survey, a rather high 220Rn progeny concentration with an average of 1.73 Bq m(-3) was observed in traditional Japanese dwellings with soil/mud plastered walls. On the other hand, a very high 232Th concentration in soil was reported in China. They suggested that there is a possibility of high 220Rn progeny concentration in both Japan and China.     

222Rn emanation from uranium-glazed ceramics

Orange-red uranium-glazed dinnerware was found to emanate 222Rn to produce an average of less than 0.1 Bq 222Rn decay per piece, which should have no associated health risks. Comparison of 222Rn emanation to 226Ra in glazes (measured by alpha spectrometry) indicated inefficient emanation (<5%) of 222Rn, consistent with the low radon levels observed and with the presence of 222Rn progeny in glazes. These studies also showed that reagent grade uranium compounds may emanate measurable 222Rn.     

广州市室内222Rn、220Rn浓度调查

目的了解广州市室内222Rn、220Rn浓度及所致居民剂量.方法于1997年11月至1998年2月期间采用CR-39 α固体径迹探测器测量了广州市33间建筑物室内累积222Rn浓度16问建筑物室内累积220Rn浓度.结果 222Rn浓度范围为3.3～238.2 Bq/m3,平均值为(79.1±56.6)Bq/m36.220Pn浓度范围为46.6～531.0 Bq/m3,平均值为(190.8±163.4)Bq/m3.结论各类建筑物室内222Rn浓度存在显著性差异.     

Biological variability influencing lung dosimetry for inhaled 222Rn and 220Rn decay products

Particle deposition, clearance and dosimetry of inhaled short-lived 222Rn and 220Rn decay products in the human respiratory tract have been modeled by a stochastic compartment system, based on an already existing deterministic model (Ho82a). In order to allow for statistical uncertainties and biological variabilities, input parameters and transfer coefficients were described by truncated lognormal frequency distributions. Applying Monte Carlo techniques, a set of parameter values is selected randomly in an iterative manner from these prespecified distributions, yielding finally basal-cell doses as probability density distributions instead of single mean doses. The resulting highly skewed dose distributions illustrate the fact that a small percentage of individuals in an exposed population receives considerably higher doses than indicated by a deterministic mean value.     

Recent Swedish experiences in 222Rn control

Swedish local authorities are responsible for decreasing 222Rn progeny concentrations in homes in their municipalities. To obtain an overall view of their experiences, concerned national authorities sent a questionnaire in 1986 to local authorities. The results were intended to form one basis for decisions by the government regarding revised statements on financial contributions, limits, etc. The results were also intended to be of use to national authorities in determining limits and recommendations and to local authorities in their field work. One result of the survey was an enhanced interest in the Rn problem among Swedish politicians and the mass media. This increased attention resulted in new plans for continued work to decrease Rn levels indoors during 1987-1989, on both a national and a local level. The experiences of the local authorities show that Rn progeny concentrations decreased to below the design level in 95% of newly built houses investigated. It was also found that Rn progeny concentrations were below the limit for reconstruction in 53% of existing homes that previously had levels exceeding the limit.